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Numerical analysis of mass transfer in packed-bed reactors with irregular particle arrangements
Ist Teil von
Chemical engineering science, 2012-10, Vol.81, p.77-83
Ort / Verlag
Kidlington: Elsevier Ltd
Erscheinungsjahr
2012
Link zum Volltext
Quelle
Elsevier ScienceDirect Journals Complete
Beschreibungen/Notizen
Packed bed reactors with moderate tube-to-particle diameter ratios are studied numerically using the computational fluid dynamics approach. Irregular particle arrangements within the reactors are generated by a modified ballistic deposition method. The study is focused on mass transfer phenomena in the reactors, while two different case studies are selected for numerical analysis, basically imitating the relevant experimental procedures. The first one is the dissolution of benzoic acid particles in water, the second one is the sublimation of naphthalene particles in air. To validate the simulation results, experimental mass transfer correlations from literature are used and a good agreement between numerical and experimental results is found. The numerical analysis provides useful data that can be applied for the improvement of the packed bed performance as well as for a deeper understanding of the fundamental transport phenomena in such reactors.
► A detailed CFD model is developed to capture mass transfer in packed bed reactors. ► Proposed model is validated against two different case studies and literature data. ► Regions with low mass transfer rate are identified based on the local hydrodynamics. ► A methodology is proposed for the numerical estimation of mass transfer coefficient.