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Plasma catalytic conversion of methane into syngas: the combined effect of discharge activation and catalysis
Ist Teil von
Catalysis today, 2004-02, Vol.89 (1), p.21-25
Ort / Verlag
Amsterdam: Elsevier B.V
Erscheinungsjahr
2004
Link zum Volltext
Quelle
Elsevier ScienceDirect Journals Complete
Beschreibungen/Notizen
In the current study we investigate the combined operation of a dielectric barrier discharge and an α-alumina supported Ni catalyst in the partial oxidation of methane. In order to separate the effects of plasma activation from catalytic processes, the study includes both purely catalytic and plasma-activated operation of the reactor. Whereas the catalyst alone is only active above 300
°C, plasma induced partial oxidation of methane is observed in the entire temperature range investigated (100–400
°C). By comparing the reaction over the Ni catalyst in different oxidation states with the catalyst support only, conclusions are drawn regarding surface and gas phase processes.