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Polymers under nanoconfinement: where are we now in understanding local property changes?

Chemical Society reviews, 2021-07, Vol.5 (14), p.85-866

Roth, Connie B

2021

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Local glass transition temperature Tg(z) of polystyrene next to different polymers: Hard vs. soft confinement

The Journal of chemical physics, 2017-05, Vol.146 (20), p.203307-203307

2017

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Two simultaneous mechanisms causing glass transition temperature reductions in high molecular weight freestanding polymer films as measured by transmission ellipsometry

Physical review letters, 2011-11, Vol.107 (23), p.235701-235701, Article 235701

2011

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Optimizing the Grafting Density of Tethered Chains to Alter the Local Glass Transition Temperature of Polystyrene near Silica Substrates: The Advantage of Mushrooms over Brushes

ACS macro letters, 2018-02, Vol.7 (2), p.269-274

2018

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Review and reproducibility of forming adsorbed layers from solvent washing of melt annealed films

Soft matter, 2020-06, Vol.16 (23), p.5366-5387

2020

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Physical Aging of Polymer Films Quenched and Measured Free-Standing via Ellipsometry: Controlling Stress Imparted by Thermal Expansion Mismatch between Film and Support

Macromolecules, 2013-12, Vol.46 (23), p.9455-9463

2013

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Experimental study of substrate roughness on the local glass transition of polystyrene

The Journal of chemical physics, 2020-06, Vol.152 (24), p.244901-244901

2020

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Polymer Glasses

1, 2017

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Physical Aging in Ultrathin Polystyrene Films: Evidence of a Gradient in Dynamics at the Free Surface and Its Connection to the Glass Transition Temperature Reductions

Macromolecules, 2010-10, Vol.43 (19), p.8296-8303

2010

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Glass transition and chain mobility in thin polymer films

Journal of electroanalytical chemistry (1992), 2005-10, Vol.584 (1), p.13-22

2005

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Forming denser glasses on soft substrates

Nature materials, 2024-05, Vol.23 (5), p.587-588

Roth, Connie B

2024

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Eliminating the Enhanced Mobility at the Free Surface of Polystyrene: Fluorescence Studies of the Glass Transition Temperature in Thin Bilayer Films of Immiscible Polymers

Macromolecules, 2007-04, Vol.40 (7), p.2568-2574

2007

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Effect of nanoscale confinement on the glass transition temperature of free-standing polymer films: Novel, self-referencing fluorescence method

Journal of polymer science. Part B, Polymer physics, 2008-12, Vol.46 (24), p.2754-2764

2008

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Gradient in refractive index reveals denser near free surface region in thin polymer films

The Journal of chemical physics, 2021-10, Vol.155 (14), p.144901-144901

2021

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Local glass transition temperature T g(z) of polystyrene next to different polymers: Hard vs. soft confinement

The Journal of chemical physics, 2017-05, Vol.146 (20), p.203307

2017

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Temperature dependent perylene fluorescence as a probe of local polymer glass transition dynamics

Soft matter, 2022-08, Vol.18 (32), p.694-614

2022

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Changes in the temperature-dependent specific volume of supported polystyrene films with film thickness

The Journal of chemical physics, 2016-06, Vol.144 (23), p.234903-234903

2016

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Development of broad modulus profile upon polymer-polymer interface formation between immiscible glassy-rubbery domains

Proceedings of the National Academy of Sciences - PNAS, 2024-01, Vol.121 (1), p.e2312533120

2024

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Comparing the impact of different adsorbed layers on the local glass transition of polymer matrices

The Journal of chemical physics, 2024-01, Vol.160 (4)

2024

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Comparing refractive index and density changes with decreasing film thickness in thin supported films across different polymers

The Journal of chemical physics, 2020-07, Vol.153 (4), p.044902-044902

2020

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Comparison of Critical Micelle Concentrations of Gradient Copolymer and Block Copolymer in Homopolymer: Novel Characterization by Intrinsic Fluorescence

Macromolecules, 2007-08, Vol.40 (16), p.5631-5633

2007

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Local Glass Transition Temperature T g(z) Within Polystyrene Is Strongly Impacted by the Modulus of the Neighboring PDMS Domain

ACS macro letters, 2020-11, Vol.9 (11), p.1625-1631

2020

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End-Tethered Chains Increase the Local Glass Transition Temperature of Matrix Chains by 45 K Next to Solid Substrates Independent of Chain Length

ACS macro letters, 2023-01, Vol.12 (1), p.1-7

2023

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Unexpected Molecular Weight Dependence to the Physical Aging of Thin Polystyrene Films Present at Ultra‐High Molecular Weights

Journal of polymer science. Part B, Polymer physics, 2019-09, Vol.57 (18), p.1224-1238

2019

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Above, below, and in-between the two glass transitions of ultrathin free-standing polystyrene films: Thermal expansion coefficient and physical aging

Journal of polymer science. Part B, Polymer physics, 2015-01, Vol.53 (1), p.64-75

2015

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Polymers under nanoconfinement: where are we now in understanding local property changes?

Local glass transition temperature Tg(z) of polystyrene next to different polymers: Hard vs. soft confinement

Two simultaneous mechanisms causing glass transition temperature reductions in high molecular weight freestanding polymer films as measured by transmission ellipsometry

Optimizing the Grafting Density of Tethered Chains to Alter the Local Glass Transition Temperature of Polystyrene near Silica Substrates: The Advantage of Mushrooms over Brushes

Review and reproducibility of forming adsorbed layers from solvent washing of melt annealed films

Physical Aging of Polymer Films Quenched and Measured Free-Standing via Ellipsometry: Controlling Stress Imparted by Thermal Expansion Mismatch between Film and Support

Experimental study of substrate roughness on the local glass transition of polystyrene

Polymer Glasses

Physical Aging in Ultrathin Polystyrene Films: Evidence of a Gradient in Dynamics at the Free Surface and Its Connection to the Glass Transition Temperature Reductions

Glass transition and chain mobility in thin polymer films

Forming denser glasses on soft substrates

Eliminating the Enhanced Mobility at the Free Surface of Polystyrene: Fluorescence Studies of the Glass Transition Temperature in Thin Bilayer Films of Immiscible Polymers

Effect of nanoscale confinement on the glass transition temperature of free-standing polymer films: Novel, self-referencing fluorescence method

Gradient in refractive index reveals denser near free surface region in thin polymer films

Local glass transition temperature T g(z) of polystyrene next to different polymers: Hard vs. soft confinement

Temperature dependent perylene fluorescence as a probe of local polymer glass transition dynamics

Changes in the temperature-dependent specific volume of supported polystyrene films with film thickness

Development of broad modulus profile upon polymer-polymer interface formation between immiscible glassy-rubbery domains

Comparing the impact of different adsorbed layers on the local glass transition of polymer matrices

Comparing refractive index and density changes with decreasing film thickness in thin supported films across different polymers

Comparison of Critical Micelle Concentrations of Gradient Copolymer and Block Copolymer in Homopolymer: Novel Characterization by Intrinsic Fluorescence

Local Glass Transition Temperature T g(z) Within Polystyrene Is Strongly Impacted by the Modulus of the Neighboring PDMS Domain

End-Tethered Chains Increase the Local Glass Transition Temperature of Matrix Chains by 45 K Next to Solid Substrates Independent of Chain Length

Unexpected Molecular Weight Dependence to the Physical Aging of Thin Polystyrene Films Present at Ultra‐High Molecular Weights

Above, below, and in-between the two glass transitions of ultrathin free-standing polystyrene films: Thermal expansion coefficient and physical aging

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