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The presentation of multimodal sensory theory and the continuous development of virtual reality technology provide new ideas and methods for the teaching reform of experimental education in colleges and universities. On the basis of defining the core concepts of multimodal sensory theory and virtual reality technology, this paper constructs a virtual simulation software development framework based on multimodal sensory theory, expounds its key technologies, and tries to develop a series of visual, operable, understandable, and interactive virtual simulation software under the guidance of multimodal sensory theory and uses deep learning algorithm to quantify and visually analyze the data of users’ behavior, emotion and cognitive engagement, and diagnose and evaluate users’ learning engagement and concentration, which effectively promote the reform of virtual reality education.