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10-Years assessment of 7 Be and 210 Pb in atmospheric bulk depositions in Cienfuegos (Cuba)
Ist Teil von
Journal of environmental radioactivity, 2022-05, Vol.246, p.106831
Ort / Verlag
England
Erscheinungsjahr
2022
Quelle
MEDLINE
Beschreibungen/Notizen
10-years records of monthly bulk atmospheric fluxes of
Be and
Pb (wet + dry, n = 119 samples) at a coastal station in Cienfuegos (Cuba) between 2010 and 2019 were reported and assessed in function of their temporal variability and meteorological influence. Fluxes of
Be and
Pb ranged from 120 to 15617 and from 29 to 911 mBq m
day
, respectively. Both radionuclides exhibited a similar seasonal trend with highest values during wet months and minimum values during dry months. The removal of
Be and
Pb from the atmosphere was mainly controlled by wet depositions, while dry deposition was estimated to be more important for
Pb (29% of the total bulk deposition) than for
Be (12%). The
Pb/
Be ratios (average of 0.10) showed low variability during wet months with abrupt peaks in the driest months with low temperatures and the highest wind speed and pressure, which was mainly attributed to contributions from soil resuspension. The calculated total deposition velocity of aerosols derived from
Be (average of 0.48 cm s
) and
Pb (average of 0.47 cm s
) was in agreement with values reported in the literature. Multiple linear regression models for the monthly fluxes of
Be and
Pb based on precipitation, temperature and pressure and explaining about 60% of their variances were derived, highlighting the preponderant role of the local and regional conditions on the variability of these radionuclides. The annual fluxes of
Be (209-1901 Bq m
y
) and
Pb (35-123 Bq m
y
) were in the range of variations observed in other coastal stations worldwide, showing fluctuations affected by changes in the amount of precipitation during the wet periods.
Be annual variability also evidenced a significant modulation with the solar activity.