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Studies on the rain scavenging process of tritium in a tropical site in India
Ist Teil von
Journal of environmental radioactivity, 2012-02, Vol.104, p.7-13
Ort / Verlag
Kidlington: Elsevier Ltd
Erscheinungsjahr
2012
Quelle
MEDLINE
Beschreibungen/Notizen
This study presents the results of one of the first systematic experiments on tritium (
3H) concentrations in ground level air against that in rainwater near a pressurized heavy water reactor in a tropical region. The samples were collected over the rainy season of three years (2007, 2008 and 2010). For this study, 31 data sets were collected and interpreted based on the theoretical information available in the literature. The specific activity ratio of
3H between rainwater and air moisture at ground level was calculated for each data set. The average specific activity ratio was found to be 1.96 ± 2.72. A correlation (
r = 0.82,
p < 0.001) was observed between the total rain hours in a day and the rainwater
3H activity. Higher rain duration with slower rain rate yielded higher
3H concentrations as more time was available for the scavenging/wash out process to take effect together with lower dilution. The present data also suggested the need to further investigate the influence of raindrop distribution and other local meteorological parameters on the
3H wash out process. An attempt was also made to predict the
3H concentration in air moisture samples using a Gaussian plume dispersion model and the values were compared with the measured
3H activity. The measured values were generally lower than the predictions.
► Studies on ground level air & rainwater
3H near a PHWR in tropical region. ► Studies on understanding the HTO wash out process in a tropical region. ► Influence of total rain hours in a day on the rainwater
3H activity was studied. ► A wide variation in specific activity ratio for
3H was observed.