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Influence on the levels of PAHs and methylated PAHs in surface soil from pollution control in China: Evidence in 2019 data compared with 2005 and 2012 data
Ist Teil von
The Science of the total environment, 2023-06, Vol.877, p.162718-162718, Article 162718
Ort / Verlag
Netherlands: Elsevier B.V
Erscheinungsjahr
2023
Quelle
Elsevier ScienceDirect Journals
Beschreibungen/Notizen
To comprehensively clarify the pollution characteristics of persistent toxic substances, the Soil and Air Monitoring Program Phase III (SAMP-III) was conducted in 2019 in China. In total, 154 surface soil samples were collected across China, and 30 unsubstituted polycyclic aromatic hydrocarbons (U-PAHs) and 49 methylated PAHs (Me-PAHs) were analyzed in this study. The mean concentrations of total U-PAHs and Me-PAHs were 540 ± 778 and 82.0 ± 132 ng/g dw, respectively. Northeastern China and Eastern China are the two regions of concern with high PAH and BaP equivalency levels. Compared with SAMP-I (2005) and SAMP-II (2012), an obvious upward temporal trend followed by a downward trend of PAH levels was observed in the past 14 years for the first time. The mean concentrations of 16 U-PAHs were 377 ± 716, 780 ± 1010, and 419 ± 611 ng/g dw in surface soil across China for the three phases, respectively. Considering rapid economic growth and energy consumption, an increasing trend from 2005 to 2012 was expected. From 2012 to 2019, the PAH levels in soils across China decreased by 50 %, which was consistent with the decline in PAH emissions. The period of reduction of PAHs in surface soil coincided with the implementation of Air and Soil Pollution Control Actions in China after 2013 and 2016, respectively. Along with the pollution control actions in China, the pollution control of PAHs and the increase in soil quality can be expected in the near future.
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•30 U-PAHs and 49 Me-PAHs were analyzed in surface soil across China in 2019.•Descending spatial trend from east to west and from north to south was observed.•From 2005 to 2019, an obvious upward followed by a downward trend was observed.•Reduction of PAHs could be caused Air and Soil Pollution Control Actions in China.