Details

Autor(en) / Beteiligte

• Lu, Meng
• Zhang, Mi
• Liu, Jiang
• Chen, Yifa
• Liao, Jia‐Peng
• Yang, Ming‐Yi
• Cai, Yue‐Peng
• Li, Shun‐Li
• Lan, Ya‐Qian

Titel

Covalent Organic Framework Based Functional Materials: Important Catalysts for Efficient CO2 Utilization

Ist Teil von

• Angewandte Chemie International Edition, 2022-04, Vol.61 (15), p.e202200003-n/a

Auflage

International ed. in English

Ort / Verlag

Weinheim: Wiley Subscription Services, Inc

Erscheinungsjahr

2022

Quelle

Alma/SFX Local Collection

Beschreibungen/Notizen

• As hot topics in the chemical conversion of CO2, the photo‐/electrocatalytic reduction of CO2 and use of CO2 as a supporter for energy storage have shown great potential for the utilization of CO2. However, many obstacles still exist on the road to realizing highly efficient chemical CO2 conversion, such as inefficient uptake/activation of CO2 and mass transport in catalysts. Covalent organic frameworks (COFs), as a kind of porous material, have been widely explored as catalysts for the chemical conversion of CO2 owing to their unique features. In particular, COF‐based functional materials containing diverse active sites (such as single metal sites, metal nanoparticles, and metal oxides) offer great potential for realizing CO2 conversion and energy storage. This Minireview discusses recent breakthroughs in the basic knowledge, mechanisms, and pathways of chemical CO2 conversion strategies that use COF‐based functional catalysts. In addition, the challenges and prospects of COF‐based functional catalysts for the efficient utilization of CO2 are also introduced. This Minireview discusses recent developments in the basic knowledge, mechanisms, and CO2 utilization strategies regarding the use of functional materials based on covalent‐organic frameworks (COFs) with diverse active sites as catalysts. Insight is provided into the challenges and prospects of COF‐based catalysts for the design of the next‐generation photo‐/electrocatalysts for the utilization of CO2.