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We report a novel plastic deformation mechanism of bulk metallic glass composites (BMGCs) containing metastable β − Ti dendrites. Plastic deformation of the BMGCs beyond the ultimate tensile strength is mediated by cooperative shear events, which comprise a shear band in the glassy matrix and a continuous ω − Ti band with a thickness of ∼ 10 nm in the β − Ti dendrite. The cooperative shear leads to serrated shear avalanches. The formation of narrow ω − Ti bands is caused by high local strain rates during the cooperative shear. The cooperative shear mechanism enriches the deformation mechanisms of BMGCs and also deepens the understanding of ω − Ti formation.