Details

Autor(en) / Beteiligte

• Platis, Andreas
• Altstädter, Barbara
• Wehner, Birgit
• Wildmann, Norman
• Lampert, Astrid
• Hermann, Markus
• Birmili, Wolfram
• Bange, Jens

Titel

Observational Case Study on the Influence of Atmospheric Boundary-Layer Dynamics on New Particle Formation

Ist Teil von

• Boundary-layer meteorology, 2016-01, Vol.158 (1), p.67-92

Ort / Verlag

Dordrecht: Springer Netherlands

Erscheinungsjahr

2016

Quelle

Alma/SFX Local Collection

Beschreibungen/Notizen

• We analyze the influence of atmospheric boundary-layer development on new particle formation (NPF) during the morning transition. Continuous in-situ measurements of vertical profiles of temperature, humidity and aerosol number concentrations were quasi-continously measured near Melpitz, Germany, by unmanned aerial systems to investigate the potential connection between NPF and boundary-layer dynamics in the context of turbulence, temperature and humidity fluctuations. On 3 April 2014 high number concentrations of nucleation mode particles up to [Formula: see text] were observed in an inversion layer located about 450 m above ground level. The inversion layer exhibited a spatial temperature structure parameter [Formula: see text] 15 times higher and a spatial humidity structure parameter [Formula: see text] 5 times higher than in the remaining part of the vertical profile. The study provides hints that the inversion layer is responsible for creating favorable thermodynamic conditions for a NPF event. In addition, this layer showed a strong anti-correlation of humidity and temperature fluctuations. Using estimates of the turbulent mixing and dissipation rates, it is concluded that the downward transport of particles by convective mixing was also the reason of the sudden increase of nucleation mode particles measured on ground. This work supports the hypothesis that many of the NPF events that are frequently observed near the ground may, in fact, originate at elevated altitude, with newly formed particles subsequently being mixed down to the ground.