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Design and Fabrication of Plasmonic Nanostructures with DNA for Surface-Enhanced Raman Spectroscopy Applications
Ist Teil von
Chinese journal of chemistry, 2016-03, Vol.34 (3), p.273-282
Ort / Verlag
Weinheim: WILEY-VCH Verlag
Erscheinungsjahr
2016
Quelle
Wiley Online Library - AutoHoldings Journals
Beschreibungen/Notizen
Plasmonic nanostructures display unique and strongly enhanced optical properties, therefore hold great promise for a wide range of spectroscopic applications, particularly surface-enhanced Raman spectroscopy (SERS). It is well acknowledged that the major contributions to SERS arise from molecules positioned in nanojunctions where the op- tical field is intensively concentrated due to localized surface plasmon excitations. One of the key challenges in SERS therefore lies in the design and fabrication of plasmonic nanostructures with controllable nanojunctions. In recent years, by exploiting the unparalleled base-pairing self-recognition properties, DNA-mediated assembly has emerged as a powerful and programmable tool for the accurate construction of complex and hierarchical plasmonic nanostructures with well-defined geometry and topology. In this review, we will summarize recent advances on de- sign and fabrication of a rich variety of plasmonic nanostructures by virtue of DNA nanotechnology, and discuss their optical properties as well as applications in SERS.