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Magnetic correlations in the semimetallic hyperkagome iridate Na3Ir3 O8
Ist Teil von
Physical review. B, 2021-03, Vol.103 (10), p.1
Ort / Verlag
College Park: American Physical Society
Erscheinungsjahr
2021
Quelle
APS_美国物理学会期刊
Beschreibungen/Notizen
We present a microscopic study of a doped quantum spin liquid candidate, the hyperkagome Na3 Ir3 O8 compound, by using 23Na NMR. We determine the intrinsic behavior of the uniform q = 0 susceptibility via shift measurements and the dynamical response by probing the spin-lattice relaxation rate. Throughout the studied temperature range, the susceptibility is consistent with a semimetal behavior, though with electronic bands substantially modified by correlations. Remarkably, the antiferromagnetic fluctuations present in the insulating parent compound Na4 Ir3 O8 survive in the studied compound. The spin dynamics are consistent with 120 ∘ excitation modes displaying short-range correlations.