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Journal of materials science. Materials in electronics, 2019-08, Vol.30 (16), p.15636-15645
2019
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Autor(en) / Beteiligte
Titel
A novel synthesis method for Ag/g-C3N4 nanocomposite and mechanism of enhanced visible-light photocatalytic activity
Ist Teil von
  • Journal of materials science. Materials in electronics, 2019-08, Vol.30 (16), p.15636-15645
Ort / Verlag
New York: Springer US
Erscheinungsjahr
2019
Quelle
SpringerLink
Beschreibungen/Notizen
  • A novel synthesis approach toward Ag/g-C 3 N 4 composite photocatalyst is reported. First, g-C 3 N 4 nanoflakes (CNNs) were fabricated by thermal polymerization of melamine precursor combined with gas bubble exfoliation method. Second, Ag nanoparticles were homogeneously dispersed on CNNs by photo-reduction method to assemble Ag/CNNs nanocomposites. The structure of Ag/CNNs nanocomposites was verified by SEM, EDS, TEM, FTIR and XRD. The photocatalytic properties of Ag/CNNs nanocomposites were verified by degradation of Rhodamine B (RhB) under visible light irradiation. The increase of photocatalytic activity of Ag/CNNs nanocomposites was mainly due to the Schottky barrier between Ag and CNNs and the local surface plasmonic resonance (LSPR) effect of Ag NPs, which was conducive to improving the separation and transportation efficiency of photogenerated electrons-holes as well as the absorption of visible light, reducing recombination of free charges. Thus, the Ag/CNNs nanocomposites would show excellent photocatalytic activity in organic waste water treatment.

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