Details

Autor(en) / Beteiligte

• Pásztorová, J.
• Howell, A.
• Songvilay, M.
• Sarte, P. M.
• Rodriguez-Rivera, J. A.
• Arévalo-López, A. M.
• Schmalzl, K.
• Schneidewind, A.
• Dunsiger, S. R.
• Singh, D. K.
• Petrovic, C.
• Hu, R.
• Stock, C.

Titel

Relaxing Kondo-screened Kramers doublets in CeRhSi3

Ist Teil von

• Physical review. B, 2019-03, Vol.99 (12)

Ort / Verlag

United States: American Physical Society (APS)

Erscheinungsjahr

2019

Quelle

American Physical Society

Beschreibungen/Notizen

• ${\mathrm{CeRhSi}}_{3}$ is a superconductor under pressure coexisting with a weakly antiferromagnetic phase characterized by a Bragg peak at q→0 = (~ 0.2,0,0.5) [N. Aso et al., J. Magn. Magn. Mater. 310, 602 (2007)]. The compound is also a heavy-fermion material with a large specific heat coefficient ${\gamma}=110$ mJ ${\mathrm{mol}}^{{-}1}{\mathrm{K}}^{{-}2}$ and a high Kondo temperature of ${T}_{K}=50$ K, indicating ${\mathrm{CeRhSi}}_{3}$ is in a strongly Kondo screened state. We apply high-resolution neutron spectroscopy to investigate the magnetic fluctuations in the normal phase, at ambient pressures, and at low temperatures. We measure a commensurate dynamic response centered around the Q→ = (0,0,2) position that gradually evolves to $H{\sim}0.2$ with decreasing temperature and/or energy transfers. The response is broadened both in momentum and energy and is not reminiscent of sharp spin wave excitations found in insulating magnets where the electrons are localized. We parametrize the excitation spectrum and temperature dependence using a heuristic model utilizing the random-phase approximation to couple relaxing ${\mathrm{Ce}}^{3+}$ ground-state Kramers doublets with a Kondo-like dynamic response. With a Ruderman-Kittel-Kasuya-Yosida exchange interaction within the $ab$ plane and an increasing single-site susceptibility, we can qualitatively reproduce the neutron spectroscopic results in ${\mathrm{CeRhSi}}_{3}$ and, namely, the trade-off between scattering at commensurate and incommensurate positions. We suggest that the antiferromagnetic phase in ${\mathrm{CeRhSi}}_{3}$ is driven by weakly correlated relaxing localized Kramers doublets and that ${\mathrm{CeRhSi}}_{3}$ at ambient pressures is on the border between a Rudderman-Kittel-Yosida antiferromagnetic state and a Kondo-screened phase where static magnetism is predominately absent.