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Distribution of neptunium and plutonium in New Mexico lichen samples (Usnea arizonica) contaminated by atmospheric fallout
Ist Teil von
Journal of radioanalytical and nuclear chemistry, 2016-03, Vol.307 (3), p.2079-2084
Ort / Verlag
Dordrecht: Springer Netherlands
Erscheinungsjahr
2016
Quelle
Alma/SFX Local Collection
Beschreibungen/Notizen
The concentrations of
237
Np,
239
Pu and
240
Pu were determined in lichen samples (
Usnea arizonica
) that were collected from ten locations in New Mexico between 2011 and 2013 using isotope dilution inductively-coupled plasma mass spectrometry (ID-ICP-MS). The observed isotopic ratios for
237
Np/
239
Pu and
240
Pu/
239
Pu indicate trace contamination from global and regional fallout (e.g. Trinity test and atmospheric testing at the Nevada Test Site). The fact that actinide contamination is detected in recent lichen collections suggests continuous re-suspension of fallout radionuclides even 50 years after ratification of the Limited Test Ban Treaty.