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Improvement of $^{93m}$Nb and $^{93m}$Rh activity measurement methodology for reactor dosimetry
Ist Teil von
EPJ Web of conferences, 2017, Vol.153
Ort / Verlag
EDP Sciences
Erscheinungsjahr
2017
Link zum Volltext
Quelle
Free E-Journal (出版社公開部分のみ)
Beschreibungen/Notizen
Reactor dosimetry is based on the analysis of the activity of irradiated dosimeters, such as $^{93m}$Nb and $^{103m}$Rh. The activity measurement of these dosimeters is conventionally performed by X-ray spectrometry, but the low-energy of emitted photons makes it difficult to derive reliable results with low uncertainties. Approaches to improve these characterisations are presented: they include high accuracy efficiency calibration of a HPGe detector using both experiments and Monte Carlo simulation, calculation of corrective factors for the geometry (selfabsorption) and self-fluorescence effects. Improvement of the knowledge of the $^{103m}$Rh decay scheme is also required and a specific experiment is proposed, including activity measurement of a $^{103m}$Rh solution by liquid scintillation, and measurement of the photon emission intensities by X-ray spectrometry. A method for calculating coefficients to take into account the self-fluorescence effects in dosimeters is also suggested to improve the uncertainties on activity measurements.