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Ionization cross of small cationic carbon clusters in high-energy collisions with helium atoms and stabilité of multiply charged species
Ist Teil von
Physical review. A, Atomic, molecular, and optical physics, 2005, Vol.72
Ort / Verlag
American Physical Society
Erscheinungsjahr
2005
Link zum Volltext
Quelle
PROLA
Beschreibungen/Notizen
Single, double, triple, and quadruple ionization cross sections of small cationic carbon clusters Cn+ colliding with helium atoms at a fixed velocity (2.6 atomic units) have been measured. The size ranges from n=1 to n=10 for single to triple ionization, from n=5 to n=10 for the quadruple ionization. The dependence of the cross sections with the cluster size is found to be well reproduced by predictions of the independent atom and electron (IAE) collision model. This extends the applicability of this simple model to higher n values and to a higher ionization degree than previously done [M. Chabot et al., Eur. Phys. J. D 14, 5 (2001)]. The branching ratios of multiply charged Cnq+ clusters remaining intact over a 100 ns time window have been measured (n=3-10, q=2-3). Branching ratios of nonfragmented doubly charged clusters have been interpreted on the basis of calculated internal energies of Cn2+ due to single ionization of Cn+ clusters using the IAE model. This allowed estimates of the minimum energies required to fragment these Cn2+ species to be derived.