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•Mn0.5Zn0.5Fe2O4-PbZryTi1-yO3 multiferroic fluids were prepared by the ball milling method.•The polarization intensity of PbZryTi1-yO3 particles reaches its maximum of 2.55 μC cm−2.•Aa high dielectric constant of 4.6 and a saturation polarization intensity of 15.69 nC cm-2 were obtained.•All specimens present obvious magnetodielectric response.•The maximum longitudinal magnetoelectric coupling coefficient αE33 is 11.49 V cm−1 Oe-1.
The Mn0.5Zn0.5Fe2O4-PbZryTi1-yO3 multiferroic fluids were prepared by the ball milling method, and the polarization intensities of PbZryTi1-yO3 particles on the magnetoelectric coupling (ME) effect were investigated. X-ray diffraction analysis (XRD) results indicate that the pure phase Mn0.5Zn0.5Fe2O4 and PbZryTi1-yO3 particles (y = 0, 0.25, 0.5, 0.75, and 1) were successfully prepared. When y = 0.5, the polarization intensity of PbZryTi1-yO3 particles reaches its maximum of 2.55 μC cm−2. At this time, the Mn0.5Zn0.5Fe2O4-PbZryTi1-yO3 multiferroic fluids possess a high dielectric constant of 4.6 and a saturation polarization intensity of 15.69 nC cm−2. After applying the magnetic field, it shows a better magnetodielectric response (56.12 %), while the ferroelectric properties are also significantly improved. When the polarization intensity reaches its maximum value, the maximum longitudinal magnetoelectric coupling coefficient αE33 is 11.49 V cm−1 Oe-1. It provides a new approach to achieving the strong magnetoelectric coupling effect in multiferroic fluids.