Sie befinden Sich nicht im Netzwerk der Universität Paderborn. Der Zugriff auf elektronische Ressourcen ist gegebenenfalls nur via VPN oder Shibboleth (DFN-AAI) möglich. mehr Informationen...
Optimization of the 3D battery architecture is crucial to improve the performance of microbatteries. However, such optimization is difficult and time consuming by hand for even experts. In this article, we propose a battery optimization system, which consists of an automatic geometry generator and performance simulators. The geometry generator creates feasible 3D batteries without using any human intuition and experience for the spatial arrangement of positive and negative electrodes. For quick evaluation of the internal resistance, which relates power and energy densities, we propose the transmission line model, the so-called 3D porous electrode model, as one of the performance simulators. To show the effectiveness of the optimization system, we designed the lithium-ion microbatteries. In the trade-off frontier for the internal resistance and the capacity, we successfully found a new battery architecture that has higher power and energy densities over the conventional interdigitated plates configuration.
[Display omitted]
•The automatic geometry generator created feasible 3D microbattery architectures•The use of TLM enabled quick evaluation of the internal resistance of the 3D battery•The optimization system could evaluate the performance of 200,000 3D microbatteries•The optimized battery showed better performance over the interdigitated geometry
Electrochemical Energy Storage; Energy Engineering; Energy Systems; Energy Materials