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Long-term observations of cloud condensation nuclei over the Amazon rain forest – Part 2: Variability and characteristics of biomass burning, long-range transport, and pristine rain forest aerosols
Ist Teil von
Atmospheric chemistry and physics, 2018-07, Vol.18 (14), p.10289-10331
Ort / Verlag
Katlenburg-Lindau: Copernicus GmbH
Erscheinungsjahr
2018
Quelle
EZB Electronic Journals Library
Beschreibungen/Notizen
Size-resolved measurements of atmospheric aerosol and cloud condensation nuclei (CCN) concentrations and hygroscopicity were conducted over a full seasonal cycle at the remote Amazon Tall Tower Observatory (ATTO, March 2014--February 2015). In a preceding companion paper, we presented annually and seasonally averaged data and parametrizations (Part 1; Pöhlker et al., 2016a). In the present study (Part 2), we analyze key features and implications of aerosol and CCN properties for the following characteristic atmospheric conditions: Long-range-transport (LRT) events, which frequently bring Saharan dust, African biomass smoke, and sea spray aerosols into the Amazon Basin, mostly during February to April. The LRT episodes are characterized by a dominant accumulation mode (D.sub.Ait â 80 nm, N.sub.Ait â 120 cm.sup.-3 vs. D.sub.acc â 180 nm, N.sub.acc â 310 cm.sup.-3 ), an increased abundance of dust and salt, and relatively high hygroscopicity (κ.sub.Ait â 0.18, κ.sub.acc â 0.35). The coarse mode is also significantly enhanced during these events.