Sie befinden Sich nicht im Netzwerk der Universität Paderborn. Der Zugriff auf elektronische Ressourcen ist gegebenenfalls nur via VPN oder Shibboleth (DFN-AAI) möglich. mehr Informationen...
Exploiting non-trivial spatio-temporal correlations of thermal radiation for sunlight harvesting
Ist Teil von
Journal of physics. B, Atomic, molecular, and optical physics, 2017-06, Vol.50 (12), p.124002
Ort / Verlag
IOP Publishing
Erscheinungsjahr
2017
Quelle
Alma/SFX Local Collection
Beschreibungen/Notizen
The promise of any small improvement in the performance of light-harvesting devices is sufficient to drive enormous experimental efforts. However, these efforts are almost exclusively focused on enhancing the power conversion efficiency with specific material properties and harvesting layers thickness, without exploiting the correlations present in sunlight-in part because such correlations are assumed to have a negligible effect. Here we show, by contrast, that these spatio-temporal correlations are sufficiently relevant that the use of specific detector geometries would significantly improve the performance of harvesting devices. The resulting increase in the absorption efficiency, as the primary step of energy conversion, may also act as a potential driving mechanism for artificial photosynthetic systems. Our analysis presents design guidelines for optimal detector geometries with realistic incident intensities based on current technological capabilities.