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Methane variability associated with natural and anthropogenic sources in an Australian context
Ist Teil von
Australian journal of earth sciences, 2018-07, Vol.65 (5), p.683-690
Ort / Verlag
Hoboken: Taylor & Francis
Erscheinungsjahr
2018
Quelle
Taylor & Francis
Beschreibungen/Notizen
Coal seam gas (CSG) has the potential to be a low-carbon transition fuel, but CSG fields may be a source of fugitive emissions of methane (CH
4
). We use mobile cavity ring-down spectroscopy (CRDS) measurements to attribute CH
4
concentrations to sources in southeastern Australia including CSG fields. Our study shows higher CH
4
concentration values associated with both natural and anthropogenic sources other than CSG. These include urban landfills (>320 ppm) and urban infrastructure (>17 ppm), agricultural activities (>20 ppm) and open-pit coal mines (>30 ppm). We confirm reports of increased concentration of CH
4
downwind of some parts of CSG fields (<5 ppm), but elevated concentrations are not endemic and could not be separated from contributions of natural geological seeps (>16 ppm) that form part of the background levels. While CRDS allows direct determination of CH
4
sources, repeat measurements show the strong influence of atmospheric conditions on concentration and highlight the need for methods that quantify flux.