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Soft matter, 2015-01, Vol.11 (36), p.7214-7218
2015
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Details

Autor(en) / Beteiligte
Titel
Spatial correlations of elementary relaxation events in glass-forming liquids
Ist Teil von
  • Soft matter, 2015-01, Vol.11 (36), p.7214-7218
Ort / Verlag
England
Erscheinungsjahr
2015
Quelle
Alma/SFX Local Collection
Beschreibungen/Notizen
  • The dynamical facilitation scenario, by which localized relaxation events promote nearby relaxation events in an avalanche process, has been suggested as the key mechanism connecting the microscopic and the macroscopic dynamics of structural glasses. Here we investigate the statistical features of this process via numerical simulations of a model structural glass. First we show that the relaxation dynamics of the system occurs through particle jumps that are irreversible, and that cannot be decomposed in smaller irreversible events. Then we show that each jump does actually trigger an avalanche. The characteristics of this avalanche change upon cooling, suggesting that the relaxation dynamics crossovers from a noise dominated regime, where jumps do not trigger other relaxation events, to a regime dominated by the facilitation process, where a jump triggers more relaxation events. We identify the smallest irreversible events in glass formers and investigate their correlations.
Sprache
Englisch
Identifikatoren
ISSN: 1744-683X
eISSN: 1744-6848
DOI: 10.1039/c5sm01510c
Titel-ID: cdi_crossref_primary_10_1039_C5SM01510C

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