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Anion-exchange precipitation synthesis of α-Ag2WO4/Zn–Cr layered double hydroxides composite with enhanced visible-light-driven photocatalytic activity
Ist Teil von
Separation and purification technology, 2013-12, Vol.120, p.134-140
Ort / Verlag
Elsevier B.V
Erscheinungsjahr
2013
Quelle
ScienceDirect Pay Per View(PPV) Titles
Beschreibungen/Notizen
•α-Ag2WO4/Zn–Cr LDHs was prepared by an anion-exchange precipitation method.•α-Ag2WO4 particles were highly dispersed on the surface of Zn–Cr LDHs materials.•α-Ag2WO4/Zn–Cr LDHs shows much higher activity in the photodegradation of RhB.•The photocatalytic mechanism was proposed.
In this paper, we report the obtention of α-Ag2WO4/Zn–Cr Layered Double Hydroxides (LDHs) composite via a facile anion-exchange precipitation reaction method by adding AgNO3 solution into WO42- anions intercalated Zn–Cr LDHs suspensions. X-ray diffraction, field emission scanning electronic microscope, X-ray photoelectron spectroscopy, and Fourier Transform Infrared Spectrum were used to characterize the products. It was found that α-Ag2WO4 crystals were dispersed on the surface of Zn–Cr LDHs materials on a large scale. The photocatalytic degradation studies on Rhodamine B indicate that α-Ag2WO4/Zn–Cr LDHs composite shows a higher visible-light-driven photocatalytic activity for degradation of organic pollutants than α-Ag2WO4 crystals and Zn–Cr LDHs. The possible photocatalytic mechanism is also discussed. Finally, a facile approach to fabricate novel types of visible-light-induced photocatalysts for environment treatment was discovered.