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Strongly correlated nickelate: Recent progress of synthesis and applications in artificial intelligence
Ist Teil von
Materials science in semiconductor processing, 2023-11, Vol.166, p.107735, Article 107735
Ort / Verlag
Elsevier Ltd
Erscheinungsjahr
2023
Quelle
Alma/SFX Local Collection
Beschreibungen/Notizen
Perovskite nickelates (ReNiO3) belong to the family of strongly correlated materials, the electrical properties of which are extremely sensitive to external stimuli. Nevertheless, material synthesis of ReNiO3 is challenging due to the metastability of the Ni3+ valence state. Recent years have witnessed both the exciting development in applications of correlated perovskite nickelates in memory devices and neuromorphic systems and progress in their synthesis techniques. In this paper, we review the epitaxial and non-epitaxial growth of correlated nickelates and highlight the role of heterogeneous nucleation and oxygen pressure in the material synthesis of metastable ReNiO3. We further discuss recent breakthroughs in the application of correlated nickelates in advanced memory and the neuromorphic devices regarding their underlying mechanisms including electro-thermally driven and interfacial-charge driven insulator-metal transitions, and ionic defect mediated local Mott transitions.