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Spectrum-enhanced Au@ZnO plasmonic nanoparticles for boosting dye-sensitized solar cell performance
Ist Teil von
Journal of power sources, 2018-03, Vol.380, p.142-148
Ort / Verlag
Elsevier B.V
Erscheinungsjahr
2018
Link zum Volltext
Quelle
Alma/SFX Local Collection
Beschreibungen/Notizen
Spectrum-enhanced Au@ZnO plasmonic nanoparticles (NPs) are developed for fabrication of the dye-sensitized solar cells (DSSCs), and their remarkable enhanced performances are achieved due to Surface Plasmon Resonance (SPR) effects. When being doped different blended amounts of the Au@ZnO NPs within the photoanode layers, various enhanced effects in the SPR-based DSSCs are exhibited. Compared with the power conversion efficiency (PCE, 7.50%) achieved for bare DSSC, device with doped Au@ZnO NPs of 1.93% delivers the top PCE of 8.91%, exhibiting about 20% enhancement. To elaborate the charge transfer process in the Au@ZnO NPs blended DSSCs, the photoluminescence (PL), electrochemical impedance spectra (EIS), etc are performed. We find that both the enhanced SPR absorption properties and the suppressed recombination process of charges contribute much to the improved performance of Au@ZnO-incorporated DSSCs.
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•Novel spectrum-enhanced Au@ZnO plasmonic nanoparticles are developed.•The optimized amounts of Au@ZnO are used to boost the DSSC performance.•Enhanced SPR effects increase the light harvesting abilities of plasmonic DSSCs.•Low recombination of charges is also responsible for the enhanced DSSCs.