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Molecular Beam Epitaxy Growth and Scanning Tunneling Microscopy Study of Pyrite CuSe: Films on SrTiO3
Ist Teil von
中国物理快报:英文版, 2015 (6), p.180-183
Erscheinungsjahr
2015
Quelle
Alma/SFX Local Collection
Beschreibungen/Notizen
We perform molecular beam epitaxy growth and scanning tunneling microscopy study of copper diselenide (CuSe2 ) films on SrTiO3 (001). Using a Se-rich condition, the single-phase pyrite CuSe2 grows in the Stranski-Krastanov (layer-plus-island) mode with a preferential orientation of (111). Our careful inspection of both the as-grown and post-annealed CuSe2 films at various temperatures invariably shows a Cu-terminated surface, which, depending on the annealing temperature, reconstructs into two distinct structures 2 ×√3 and √x ×√3-R30°. The Cu termi- nation is supported by the depressed density of states near the Fermi level, measured by in-situ low temperature scanning tunneling spectroscopy. Our study helps understand the preparation and surface chemistry of transition metal pyrite dichalcogenides thin films.